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Title In situ synthesis of ultrahigh molecular weight polyethylene/graphene oxide nanocomposite using the immobilized single-site catalyst
Type JournalPaper
Keywords Disentangled, immobilization, nanocomposites, single-site catalyst, ultrahigh molecular weight polyethylene
Abstract We address the immobilization of single-site catalyst on the graphite oxide (GO) surface using methylaluminoxane. Ethylene polymerization was performed using the immobilized catalyst and the nanocomposite of ultrahigh molecular weight polyethylene (UHMWPE)/GO with less entanglement density was obtained. It was observed that the drawability, mechanical and thermal properties of the produced polymer significantly are affected by the anchoring of polymer chains to the GO nanosheets. The orientation and location of crystalline lamellae and nanosheets were verified by microscopic techniques. Besides, X-ray analysis demonstrated the dispersion of GO within the UHMWPE phase and crystallinity of UHMWPE/GO nanocomposites enhanced during drawing process.
Researchers Elchin Jafariyeh-Yazdi (Fifth Researcher), Hasan Keshavarz-Mirzamohamadi (Fourth Researcher), mostafa rezaei (Third Researcher), saeid talebi (Second Researcher), Amin Heidari (First Researcher)